STUDIES ON RANDOMNESS AND NUCLEATION RATE OF SUPERCOOLED WATER FREEZING FROM HOMOGENEOUS NUCLEATION
Author(s) -
QU KAI-YANG,
JIANG YI
Publication year - 2000
Publication title -
acta physica sinica
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.199
H-Index - 47
ISSN - 1000-3290
DOI - 10.7498/aps.49.2214
Subject(s) - supercooling , nucleation , homogeneous , randomness , classical nucleation theory , thermodynamics , materials science , chemical physics , statistical physics , physics , mathematics , statistics
The dependence of the probability of the supercooled water freezing from homogeneous nucleation on the volume, time and temperature was deduced based on the “continuum” model of water structure put forward by Stanley and Teixeira. The homogeneous nucleation rate of supercooled water freezing was then calculated. The results agreed with the experimental measurements. The calculation of the pre-exponential factor, which is a key for the classical nucleation theory and the density functional method,is not needed for this method.
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