Open AccessNONLINEAR OPTICAL PROPERTIES OF THE SUBSTITU-TIONAL FULLERENE C77X(X=B,N ATOMS)
Author(s) -
Jin Zhu,
Jianji Dong,
Xiangang Wan
Publication year - 1999
Publication title -
wuli xuebao
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.199
H-Index - 47
ISSN - 1000-3290
DOI - 10.7498/aps.48.2042
Subject(s) - polarizability , fullerene , doping , dispersion (optics) , materials science , nonlinear optical , spectral line , nonlinear system , atomic physics , molecular physics , order (exchange) , condensed matter physics , physics , molecule , optics , optoelectronics , quantum mechanics , finance , economics
Using the extened Su-Schrieffer-Heeger model and the Sum-Over-State method, we have calculated the third-order nonlinear polarizability γ and its dispersion spectra for single substitutional fullerenes C77X(X=B or N atoms). The results indicate:(1) compared with C78,each of the static values of γ through the substitutional doping increases to some extent (3—40 times);(2) the dynamic nonliear optical reponse of C77X not only depends on doping atoms, but also depends on the substituted isomers and doped sites.