Open AccessINVESTIGATION OF DEGENERATE FOUR-WAVE MIXING AND PHASE CONJUGATION IN ORGANIC DYE SOLUTIONS
Author(s) -
Cunkai Wu,
Fan Jun-Yin,
Zhiying Wang
Publication year - 1981
Publication title -
wuli xuebao
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.199
H-Index - 47
ISSN - 1000-3290
DOI - 10.7498/aps.30.189
Subject(s) - degenerate energy levels , energy conversion efficiency , phase conjugation , mixing (physics) , four wave mixing , rhodamine 6g , materials science , nonlinear optics , phase (matter) , optics , analytical chemistry (journal) , physics , optoelectronics , chemistry , quantum mechanics , organic chemistry , fluorescence , laser
Phase conjugation of backward-and forward-wave produced by degenerate four-wave mixing using a nearly resonantly enhanced nonlinearity in four-level organic dye solutions was investigated. The conversion efficiency of 22% had been obtained in a 2.5 X 10-5 - molar solution of Chlorophyll A in methylalcohol with a 5 mm interaction length and a pumping energy of 8 mJ from SH of a Q-switched Nd: YAG. Degene-rate four-wave mixing by two-photon resonant-enhancement in the solution of rhodamine 6G in alcohol was studied. Measurements were performed which described the dependence of nonlinear reflectivities on the molar concentrations of the media and the intensities of the pumping and object waves. Phase conjugation characteristics of forward-wave in four-wave mixing process were theoretically analysed. Experiments have cofirmed the theoretical prediction. The method of quartet degenerate four-wave mixing had been ex-tended to the doublet degenerate case. Using this method image conversion from 1.06 μm to 5320 ? had been realized with a conversion efficiency of 25% in a 5 mm long satu-rable absorber made of organic dye 9740 solution in dichloroethane. Theoretical analy-sis showed that using a medium, which is a near resonant absorber for the infrared object wave but is transparent for the visible reconstruction wave, the conversion efficiency may be well in excess of unity.