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226 Ra determination via the rate of 222 Rn ingrowth with the Radium Delayed Coincidence Counter (RaDeCC)
Author(s) -
Geibert Walter,
Rodellas Valentí,
Annett Amber,
van Beek Pieter,
GarciaOrellana Jordi,
Hsieh YuTe,
Masque Pere
Publication year - 2013
Publication title -
limnology and oceanography: methods
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.898
H-Index - 72
ISSN - 1541-5856
DOI - 10.4319/lom.2013.11.594
Subject(s) - radium , coincidence , radiochemistry , coincidence counting , liquid scintillation counting , isotope , scintillation counter , whole body counting , radon , physics , proportional counter , radionuclide , calibration , mass spectrometry , nuclear medicine , chemistry , nuclear physics , detector , optics , medicine , alternative medicine , pathology , quantum mechanics
We present a new method to determine 226 Ra in aqueous environmental samples, based on the rate of ingrowth of 222 Rn from 226 Ra, using the radium delayed coincidence counter (RaDeCC). We use the same instrument setup that is used for the determination of 223 Ra and 224 Ra. In contrast to methods published earlier, the approach does not require a modification of the counting equipment, counting separately for 226 Ra, or waiting for radioactive equilibrium. We show that the calibration works from as low as 10 dpm (0.166 Bq) per sample, up to more than 1000 dpm (16.7 Bq). Although uncertainties are larger (typically around 10%) than reported uncertainties for γ counting, liquid scintillation, or mass spectrometry at comparable activities, the simple setup, low cost, and robustness of the method make it a useful approach for underway measurements, combinations with short‐lived radium isotopes, or monitoring purposes when limited funding or infrastructure is available.