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Nutrient and Trace Element Leaching following Mine Reclamation with Biosolids
Author(s) -
Stehouwer Richard,
Day Rick L.,
Macneal Kirsten E.
Publication year - 2006
Publication title -
journal of environmental quality
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.888
H-Index - 171
eISSN - 1537-2537
pISSN - 0047-2425
DOI - 10.2134/jeq2005.0134
Subject(s) - biosolids , land reclamation , leaching (pedology) , leachate , lysimeter , environmental science , nutrient , revegetation , environmental chemistry , water quality , environmental engineering , chemistry , soil water , soil science , ecology , organic chemistry , biology
Mine reclamation with biosolids increases revegetation success but nutrient addition well in excess of vegetation requirements has the potential to increase leaching of NO 3 and other biosolids constituents. A 3‐yr water quality monitoring study was conducted on a Pennsylvania mine site reclaimed with biosolids applied at the maximum permitted and standard loading rate of 134 Mg ha −1 Zero‐tension lysimeters were installed at 1‐m depth 1 yr before reclamation: three in the biosolids application area, one in a control area (no biosolids). Before reclamation, all water samples had pH in the range 4.7 to 6.2, acidity <20 mg L −1 , and very low levels of all other measured parameters. Following reclamation, percolate water in the biosolids‐treated area had lower pH and greater acidity than the control area. Acidity was greatest during the first winter following biosolids application, decreased during the spring, and showed a similar pattern but with much smaller concentrations the second year. Maximum first‐ year leachate NO 3 concentrations were ∼300 mg L −1 and half as large the second year. Estimated inorganic N leaching loss during the first 2 yr after biosolids application was 2327 kg N ha −1 Aluminum, Mn, Cu, Ni, Pb, and Zn followed similar leaching patterns as did acidity, and their mobilization appeared to be the result of the increased acidity. These results indicate that large applications of low‐C/N‐ratio biosolids could negatively impact area water quality and that biosolids reclamation practices should be modified to reduce this possibility.