Open AccessRapid phase-cycled two-dimensional optical spectroscopy in fluorescence and transmission mode
Author(s) -
Wolfgang Wagner,
Chunqiang Li,
John L. Semmlow,
Warren S. Warren
Publication year - 2005
Publication title -
optics express
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.394
H-Index - 271
ISSN - 1094-4087
DOI - 10.1364/opex.13.003697
Subject(s) - spectroscopy , rubidium , optics , fluorescence spectroscopy , materials science , phase (matter) , transmission (telecommunications) , time resolved spectroscopy , coherent spectroscopy , fluorescence , physics , coherent anti stokes raman spectroscopy , raman spectroscopy , raman scattering , telecommunications , potassium , quantum mechanics , computer science , metallurgy
Two dimensional magnetic and optical spectra contain information about structure and dynamics inaccessible to the linear spectroscopist. Recently, phase cycling techniques in optical spectroscopy have extended the capabilities of two-dimensional electronic spectroscopy. Here, we present a method to generate collinear pump/probe pulses at high update rates for two-dimensional electronic spectroscopy. Both fluorescence mode and transmission mode photon echo data from rubidium vapor is presented.