Rapid phase-cycled two-dimensional optical spectroscopy in fluorescence and transmission mode | Zendy

Wolfgang Wagner | Zendy; Chunqiang Li | Zendy; John L. Semmlow | Zendy; Warren S. Warren | Zendy

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Rapid phase-cycled two-dimensional optical spectroscopy in fluorescence and transmission mode

Author(s) -

Wolfgang Wagner,

Chunqiang Li,

John L. Semmlow,

Warren S. Warren

Publication year - 2005

Publication title -

optics express

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.394

H-Index - 271

ISSN - 1094-4087

DOI - 10.1364/opex.13.003697

Subject(s) - spectroscopy , rubidium , optics , fluorescence spectroscopy , materials science , phase (matter) , transmission (telecommunications) , time resolved spectroscopy , coherent spectroscopy , fluorescence , physics , coherent anti stokes raman spectroscopy , raman spectroscopy , raman scattering , telecommunications , potassium , quantum mechanics , computer science , metallurgy

Two dimensional magnetic and optical spectra contain information about structure and dynamics inaccessible to the linear spectroscopist. Recently, phase cycling techniques in optical spectroscopy have extended the capabilities of two-dimensional electronic spectroscopy. Here, we present a method to generate collinear pump/probe pulses at high update rates for two-dimensional electronic spectroscopy. Both fluorescence mode and transmission mode photon echo data from rubidium vapor is presented.

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