4D spatiotemporal evolution of combustion intermediates in turbulent flames using burst-mode volumetric laser-induced fluorescence

High-speed (20 kHz rate), volumetric laser-induced-fluorescence imaging of combustion intermediates such as a formaldehyde (CH 2 O) and polycyclic aromatic hydrocarbon (PAH) species is demonstrated for tracking the four-dimensional (4D) evolution of turbulent flames. The third-harmonic, 355 nm output of a burst-mode Nd:YAG laser with a 130 mJ/pulse is expanded to 30 mm diameter for volume illumination of the base region of a methane-hydrogen jet diffusion flame. Eight simultaneous images from different viewing angles are used to collect the resulting fluorescence signal for reconstruction of 200 time-sequential three-dimensional volumes over 10 ms duration. The signal-to-noise ratio (SNR) of 300:1 is achieved after reconstruction with a temporal resolution of 100 ns and spatial resolution of 0.85-1.5 mm.