Open AccessPhase-matching-free pulse retrieval based on transient absorption in solids
Author(s) -
Adrien Leblanc,
Philippe Lassonde,
S. Petit,
Jean-Christophe Delagnes,
Elissa Haddad,
Guilmot Ernotte,
Mina R. Bionta,
Vincent Gruson,
Bruno E. Schmidt,
Heide Ibrahim,
Éric Cormier,
François Légaré
Publication year - 2019
Publication title -
optics express
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.394
H-Index - 271
ISSN - 1094-4087
DOI - 10.1364/oe.27.028998
Subject(s) - optics , materials science , ultrashort pulse , ultrafast laser spectroscopy , optical parametric amplifier , free spectral range , femtosecond , wavelength , laser , optical amplifier , optoelectronics , physics
In this paper, we introduce a pulse characterization technique that is free of phase-matching constraints, exploiting transient absorption in solids as an ultrafast optical switch. Based on a pump-probe setup, this technique uses pump pulses of sufficient intensity to induce the switch, while the pulses to characterize are probing the transmissivity drop of the photoexcited material. This enables the characterization of low-intensity ultra-broadband pulses at the detection limit of the spectrometer and within the transparency range of the solid. For example, by using zinc selenide (ZnSe), pulses with wavelengths from 0.5 to 20 μ m can be characterized, denoting five octaves of spectral range. Using ptychography, we retrieve the temporal profiles of both the probe pulse and the switch. To demonstrate this approach, we measure ultrashort pulses from a titanium-sapphire (Ti-Sa) amplifier, which are compressed using a hollow core fiber setup, as well as infrared to mid-infrared pulses generated from an optical parametric amplifier (OPA). The characterized pulses are centered at wavelengths of 0.77, 1.53, 1.75, 4, and 10 μ m, down to sub-two optical cycles duration, exceeding an octave of bandwidth, and with energy as low as a few nanojoules.