Open Access
Routes of odd-even harmonic emission from oriented polar molecules
Author(s) -
Xuejiao Xie,
Shujuan Yu,
Weiyan Li,
Shang Wang,
Yanjun Chen
Publication year - 2018
Publication title -
optics express
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.394
H-Index - 271
ISSN - 1094-4087
DOI - 10.1364/oe.26.018578
Subject(s) - high harmonic generation , physics , ionization , electron , atomic physics , laser , quantum tunnelling , field (mathematics) , coulomb , harmonic , quantum mechanics , ion , mathematics , pure mathematics
We study odd-even high-harmonic generation (HHG) from oriented asymmetric molecules with different symmetries in strong laser fields. A model based on strong-field approximations is used which allows us to resolve the contributions of different emission routes to odd-even HHG. The comparison between the HHG yields of all routes versus one certain route demonstrates that the routes in which the electron ionizes from the gerade component of the asymmetric orbital contribute mainly to odd-even HHG. We show that the potential mechanism is associated with effects of intramolecular interference in tunneling ionization as the bound electron passes through the barrier formed by the laser field and the asymmetric Coulomb potential. The influences of different emission routes on asymmetric orbital imagining with odd-even HHG are also addressed.