Open AccessStimulated Raman scattering detection for chemically specific time-resolved imaging of gases
Author(s) -
Eynas Amer,
Per Gren,
Stefan Edenharder,
Mikael Sjödahl
Publication year - 2016
Publication title -
optics express
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.394
H-Index - 271
ISSN - 1094-4087
DOI - 10.1364/oe.24.009984
Subject(s) - optics , raman scattering , materials science , beam (structure) , wavelength , signal (programming language) , raman spectroscopy , methane , scattering , physics , chemistry , organic chemistry , computer science , programming language
A stimulated Raman scattering (SRS) imaging technique based on spatial modulation of the pump beam has been used to study gases. The SRS gain signal was separated from the Stokes beam background in the spatial frequency domain. The SRS signal shows linear behaviour with the gas pressure at a range from 1.0 to 8.0 bars. The signal is linearly proportional to the pump beam intensity while it is enhanced with increasing the Stokes beam intensity to a certain limit than it saturates. Further, the chemical specificity of the technique has been investigated. Two sharp peaks with line width at half maximum of about 0.30 nm have been obtained at Stokes beam wavelengths of 629.93 nm and 634.05 nm corresponding to the methane and ethylene gases, respectively. The results show that SRS imaging is a promising technique to provide chemical specificity as well as spatial and temporal information of gaseous species.