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Generation of intense 11-fs ultraviolet pulses using phase modulation by two types of coherent molecular motions
Author(s) -
Yuichiro Kida,
Shin Ichi Zaitsu,
Totaro Imasaka
Publication year - 2008
Publication title -
optics express
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.394
H-Index - 271
ISSN - 1094-4087
DOI - 10.1364/oe.16.013492
Subject(s) - optics , ultrashort pulse , bandwidth limited pulse , ultraviolet , pulse (music) , dispersion (optics) , phase modulation , femtosecond pulse shaping , self phase modulation , materials science , pulse shaping , phase (matter) , pulse compression , modulation (music) , multiphoton intrapulse interference phase scan , laser , physics , nonlinear optics , phase noise , telecommunications , radar , quantum mechanics , detector , computer science , acoustics
The use of two types of phase modulations arising from the coherent rotations of ortho-hydrogen and para-hydrogen to generate an intense ultrashort ultraviolet pulse without substantial generation of sub-pulses was demonstrated. This technique allows use of a high-energy long-probe pulse in the pump-probe regime for generating a high-energy compressed pulse. A 100-fs ultraviolet pulse was compressed to 11-fs by the phase modulation followed by dispersion compensation with chirped mirrors.

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