Open AccessCascaded photoenhancement from coupled nanoparticle and microcavity resonance effects
Author(s) -
Kirk A. Fuller,
David D. Smith
Publication year - 2007
Publication title -
optics express
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.394
H-Index - 271
ISSN - 1094-4087
DOI - 10.1364/oe.15.003575
Subject(s) - materials science , nanoparticle , resonance (particle physics) , resonator , absorption (acoustics) , dielectric , scattering , optics , microsphere , photoluminescence , light scattering , mie scattering , optoelectronics , nanotechnology , atomic physics , chemical engineering , composite material , physics , engineering
Calculations, based on modal analysis of scattering and absorption by compound spheres indicate that the absorption cross sections of metal nanoparticles immobilized onto dielectric microspheres can be greatly enhanced by cavity resonances in the microspheres without significant degradation of the resonators. Gain factors for optical processes associated with the nanoparticles of 10(3) 10(4) are predicted for realistic experimental conditions using homogenous microspheres. This mechanism for cascaded photoenhancement thus has the potential of dramatically increasing the sensitivities of vibrational and photoluminescent spectroscopies.