Iterative design of multilayered dielectric microspheres with tunable transparency windows

Suspensions of microparticles dispersed in air or liquids are useful for designing media with desirable optical extinction properties within the visible or infrared spectrum. We describe here a numerical iterative optimization algorithm used to design multilayered concentric dielectric spheres with prescribed optical scattering properties. Our method integrates a computationally efficient rigorous electromagnetic solver, based on Mie theory, within an optimization loop to determine specific particle configurations that best meet a desired optical response. In particular, we show that this method can be used to design all-dielectric spherical particles that possess narrow tunable transparency windows while removing any angular dependency on the optical response.