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Finding new electrolyte additives could help create lithium-ion batteries with better performance at high voltage, allowing higher energy density. However, finding the perfect additive remains a tremendous challenge, since researchers still don’t understand how to predict their performance. A new group of dioxazolone electrolyte additives have been tested in lithium-ion batteries alone or in combination with well-known co-additives. The new additives consist of a 3-phenyl-1,4,2-dioxazol-5-one (PDO) parent structure with or without (methoxy, fluoro and nitro) functional groups on the para position of the phenyl ring. It is found that PDO (no functional group) and  p -(4-nitrophenyl)-1,4,2-dioxazol-5-one (pNDO) are the best performing dioxazolones overall and show promising results.

Impact of Functionalization and Co-Additives on Dioxazolone Electrolyte Additives