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Rapid U‐Pb Geochronology by Laser Ablation Multi‐Collector ICP‐MS
Author(s) -
Sundell Kurt E.,
Gehrels George E.,
Pecha Mark E.
Publication year - 2021
Publication title -
geostandards and geoanalytical research
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.037
H-Index - 73
eISSN - 1751-908X
pISSN - 1639-4488
DOI - 10.1111/ggr.12355
Subject(s) - geochronology , zircon , laser ablation , geology , mineralogy , sample (material) , analytical chemistry (journal) , geochemistry , laser , chemistry , physics , optics , environmental chemistry , chromatography
Detrital zircon (DZ) U‐Pb laser ablation‐inductively coupled plasma‐mass spectrometry (LA‐ICP‐MS) has revolutionised the way geologists approach many Earth science questions. Although recent research has focused on rapid sample throughput, acquisition rates are limited to 100–300 analyses h −1 . We present a method to acquire zircon U‐Pb dates at rates of 120, 300, 600 and 1200 analyses h −1 (30, 12, 6 and 3 s per analysis) by multi‐collector LA‐ICP‐MS. We demonstrate the efficacy of this method by analysing twelve zircon reference materials with dates from ~ 3465 to ~ 28 Ma. Mean offset from high‐precision dates increases with faster rates from 0.9% to 1.1%; mean random 1 s uncertainty increases from 0.6% to 1.3%. We tested this new method on a sandstone sample previously characterised by large‐ n DZ geochronology. Quantitative comparison shows increased correspondence among age distributions comprising > 300 dates. This new method holds promise for DZ geochronology because (a) it requires no major changes to hardware, but rather modifications to software; (b) it yields robust age distributions well‐suited for quantitative analysis and maximum depositional age calculations; (c) there is only a minor sacrifice of accuracy and measurement uncertainty; and (d) there is less burden to researchers in terms of time investment and analytical cost.
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