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Resonant photocurrent from a single quantum emitter in tungsten diselenide
Author(s) -
Matthias Paur,
Aday J. MolinaMendoza,
Dmitry K. Polyushkin,
Steffen Michaelis de Vasconcellos,
Rudolf Bratschitsch,
Thomas Mueller
Publication year - 2020
Publication title -
2d materials
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 2.702
H-Index - 72
ISSN - 2053-1583
DOI - 10.1088/2053-1583/aba4ec
Subject(s) - tungsten diselenide , photocurrent , optoelectronics , common emitter , monolayer , photon , photon antibunching , physics , materials science , quantum optics , optics , nanotechnology , chemistry , transition metal , biochemistry , catalysis
Single quantum emitters (SQEs) are the basic building blocks for quantum optics and quantum information technology. Strain-induced defects in monolayer transition metal dichalcogenides (TMDs) have been shown to be a promising platform for the generation of SQEs. In particular, achieving optically active and electrically controlled quantum emitters make these materials attractive for applications ranging from quantum communication and optoelectronics to high resolution metrology. Here, we report the spectral photoresponse of monolayer WSe 2 upon strain, where we observe a connection between single-photon emission and photocurrent (PC) generation in a p-n device. A strong antibunching in second-order correlation from this localized emitter unambiguously demonstrates the single-photon nature of the emission, whereas the PC is highly dominated by the absorption at such a localized state, showing an exponential dependence with the applied electric field. Furthermore, we can resolve narrow PC peaks with 1.0 meV spectral width.

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