
Dynamic multifunctional devices enabled by ultrathin metal nanocoatings with optical/photothermal and morphological versatility
Author(s) -
Songshan Zeng,
Zhuoran Yang,
Zaili Hou,
Cheonjin Park,
Michael D. Jones,
Hao Ding,
Kuangyu Shen,
Andrew T. Smith,
Henry X. Jin,
Bing Wang,
Han Jiang,
Luyi Sun
Publication year - 2022
Publication title -
proceedings of the national academy of sciences of the united states of america
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 5.011
H-Index - 771
eISSN - 1091-6490
pISSN - 0027-8424
DOI - 10.1073/pnas.2118991119
Subject(s) - materials science , photothermal therapy , photothermal effect , nanotechnology , nanoscopic scale , optoelectronics
Significance Smart devices characterized by micro-/nanotopographies, such as cracks, wrinkles, folds, etc., have been fabricated for widespread application. Here, with the combination of multiscale hierarchical architecture, ultrathin metal nanocoatings with high optical/photothermal tunability and morphological versatility, and surface/interface engineering, a set of multifunctional devices with multistimuli responsiveness was fabricated. These devices can adapt to external stimuli with reversible and instantaneous responses in optical signals, which include strain-regulated light-scattering properties, photothermal-responsive wrinkled surface coupled with moisture-responsive structural color, and mechanically controllable light-shielding properties. The structural designs that rationally overlay micro-/nanostructured ultrathin nanocoatings with other elements are the key to realize this advanced system, which provides avenues for designing versatile, tunable, and adaptable multifunctional devices.