Physical origin of the third order nonlinear optical response of orthogonal pyrrolo-tetrathiafulvalene derivatives | Zendy

Konstantinos Iliopoulos | Zendy; Robert Czaplicki | Zendy; Hasnaa El Ouazzani | Zendy; JeanYves Balandier | Zendy; Marcos Chas | Zendy; Sébastien Goeb | Zendy; Marc Sallé | Zendy; Denis Gindre | Zendy; B. Sahraoui | Zendy

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Physical origin of the third order nonlinear optical response of orthogonal pyrrolo-tetrathiafulvalene derivatives

Author(s) -

Konstantinos Iliopoulos,

Robert Czaplicki,

Hasnaa El Ouazzani,

JeanYves Balandier,

Marcos Chas,

Sébastien Goeb,

Marc Sallé,

Denis Gindre,

B. Sahraoui

Publication year - 2010

Publication title -

applied physics letters

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.182

H-Index - 442

eISSN - 1077-3118

pISSN - 0003-6951

DOI - 10.1063/1.3482943

Subject(s) - tetrathiafulvalene , degenerate energy levels , nonlinear system , nonlinear optics , nonlinear optical , absorption (acoustics) , materials science , optics , molecular physics , physics , molecule , quantum mechanics

International audience

We present the third order nonlinear optical study of tetrathiafulvalene-based molecular corners. Degenerate four-wave mixing measurements have been done to provide information about the magnitude and the origin of the nonlinearity, while the nonlinear absorption has been separately measured by performing “open aperture” Z-scan measurements. The response has been found to be strongly dependent upon the structure of the molecular corners.

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