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Quantifying Nitrous Oxide Emissions in the U.S. Midwest: A Top‐Down Study Using High Resolution Airborne In‐Situ Observations
Author(s) -
Eckl Maximilian,
Roiger Anke,
Kostinek Julian,
Fiehn Alina,
Huntrieser Heidi,
Knote Christoph,
Barkley Zachary R.,
Ogle Stephen M.,
Baier Bianca C.,
Sweeney Colm,
Davis Kenneth J.
Publication year - 2021
Publication title -
geophysical research letters
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 2.007
H-Index - 273
eISSN - 1944-8007
pISSN - 0094-8276
DOI - 10.1029/2020gl091266
Subject(s) - nitrous oxide , greenhouse gas , environmental science , atmospheric sciences , nitrogen oxides , agriculture , flooding (psychology) , atmospheric chemistry , emission inventory , ecosystem , meteorology , ozone , chemistry , geography , ecology , physics , air quality index , oceanography , geology , psychology , archaeology , engineering , psychotherapist , biology , waste management , organic chemistry
Abstract The densely farmed U.S. Midwest is a prominent source of nitrous oxide (N 2 O) but top‐down and bottom‐up N 2 O emission estimates differ significantly. We quantify Midwest N 2 O emissions by combining observations from the Atmospheric Carbon and Transport‐America campaign with model simulations to scale the Emissions Database for Global Atmospheric Research (EDGAR). In October 2017, we scaled agricultural EDGAR v4.3.2 and v5.0 emissions by factors of 6.3 and 3.5, respectively, resulting in 0.42 nmol m −2 s −1 Midwest N 2 O emissions. In June/July 2019, a period when extreme flooding was occurring in the Midwest, agricultural scaling factors were 11.4 (v4.3.2) and 9.9 (v5.0), resulting in 1.06 nmol m −2 s −1 Midwest emissions. Uncertainties are on the order of 50 %. Agricultural emissions estimated with the process‐based model DayCent (Daily version of the CENTURY ecosystem model) were larger than in EDGAR but still substantially smaller than our estimates. The complexity of N 2 O emissions demands further studies to fully characterize Midwest emissions.