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Increases in aerosol concentrations over eastern China due to the decadal‐scale weakening of the East Asian summer monsoon
Author(s) -
Zhu Jianlei,
Liao Hong,
Li Jianping
Publication year - 2012
Publication title -
geophysical research letters
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 2.007
H-Index - 273
eISSN - 1944-8007
pISSN - 0094-8276
DOI - 10.1029/2012gl051428
Subject(s) - aerosol , east asian monsoon , climatology , environmental science , monsoon , east asia , atmospheric sciences , sulfate , chemical transport model , china , precipitation , geography , geology , meteorology , chemistry , archaeology , organic chemistry
China has been experiencing increased concentrations of aerosols, commonly attributed to the large increases in emissions associated with the rapid economic development. We show by using a chemical transport model driven by the assimilated meteorological fields that the observed decadal‐scale weakening of the East Asian summer monsoon also contributed to the increases in aerosols in China. We find that the simulated aerosol concentrations have strong negative correlations with the strength of the East Asian Summer monsoon. Accounting for sulfate, nitrate, ammonium, black carbon, and organic carbon aerosols, the summer surface‐layer PM 2.5 concentration averaged over eastern China (110°–125°E, 20°–45°N) can be 17.7% higher in the weakest monsoon years than in the strongest monsoon years. The weakening of the East Asian Summer monsoon increases aerosol concentrations mainly by the changes in atmospheric circulation (the convergence of air pollutants) in eastern China.