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Seasonal and latitudinal variability of troposphere Δ 14 CO 2 : Post bomb contributions from fossil fuels, oceans, the stratosphere, and the terrestrial biosphere
Author(s) -
Randerson J. T.,
Enting I. G.,
Schuur E. A. G.,
Caldeira K.,
Fung I. Y.
Publication year - 2002
Publication title -
global biogeochemical cycles
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 2.512
H-Index - 187
eISSN - 1944-9224
pISSN - 0886-6236
DOI - 10.1029/2002gb001876
Subject(s) - stratosphere , biosphere , troposphere , tundra , atmospheric sciences , environmental science , northern hemisphere , atmosphere (unit) , climatology , terrestrial ecosystem , carbon cycle , flux (metallurgy) , oceanography , geology , ecosystem , arctic , ecology , chemistry , meteorology , geography , biology , organic chemistry
During the mid‐1960s, large seasonal amplitudes were observed in surface measurements of Δ 14 C in the Northern Hemisphere. These seasonal oscillations were initially caused by stratosphere‐troposphere exchange, with the injection of bomb 14 C into the troposphere during winter and spring mixing. Here we show how fossil, ocean, and terrestrial biosphere fluxes modified the stratospheric signal during the 1960s, and the evolution of each of these components in the post bomb era. In our analysis, we used the Goddard Institute for Space Studies (GISS) atmospheric tracer model, gross ocean CO 2 fluxes from the Lawrence Livermore National Laboratory (LLNL) ocean model, and terrestrial CO 2 fluxes from a biosphere‐atmosphere model driven by normalized difference vegetation index and surface air temperatures. We found that 14 C‐depeleted respiration from the terrestrial biosphere partially canceled the 14 C‐enriched stratosphere flux in the Northern Hemisphere in the mid and late 1960s. In more recent decades, our analysis suggested that the terrestrial biosphere contribution to the Δ 14 C seasonal cycle reversed phase, with the terrestrial biosphere currently releasing relatively 14 C‐enriched CO 2 that mixes with relatively depleted troposphere CO 2 . The timing of this reversal depended on the residence times of carbon within the footprint of the observation station. Measurements of Δ 14 C in respiration from tundra and boreal ecosystems in Alaska provide evidence that some boreal forests have undergone this transition, while some tundra ecosystems have not. We predict that over the next century, several features of the latitudinal profile of Δ 14 C will substantially change because of continued fossil fuel emissions in the Northern Hemisphere, and the partial release of bomb 14 C that has accumulated in Southern Hemisphere oceans.