High-Entropy Perovskite Fluorides: A New Platform for Oxygen Evolution Catalysis
Author(s) -
Tao Wang,
Hao Chen,
Zhenzhen Yang,
Jiyuan Liang,
Sheng Dai
Publication year - 2020
Publication title -
journal of the american chemical society
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 7.115
H-Index - 612
eISSN - 1520-5126
pISSN - 0002-7863
DOI - 10.1021/jacs.9b12377
Subject(s) - chemistry , catalysis , oxygen evolution , perovskite (structure) , electrocatalyst , oxygen , mechanochemistry , entropy (arrow of time) , chemical engineering , inorganic chemistry , nanotechnology , thermodynamics , organic chemistry , electrochemistry , physics , materials science , electrode , engineering
High-entropy perovskite fluorides (HEPFs) have great potential in electrocatalysis that has not been realized because of the limitation of a high-temperature synthetic route and the limited understanding of high-entropy materials. The use of HEPFs in effective oxygen evolution catalysis and a feasible synthesis route for HEPFs in a boiled solution by combining a hydrothermal method with mechanochemistry are first reported here. These HEPFs consisting of cost-effective elements dramatically gave excellent catalytic activity for the oxygen evolution reaction in an alkaline media.
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