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Larger Stabilizing Particles Make Stronger Liquid Marble
Author(s) -
Liu Zhou,
Zhang Yuyan,
Chen Chengliu,
Yang Tiyun,
Wang Jidong,
Guo Ling,
Liu Peng,
Kong Tiantian
Publication year - 2019
Publication title -
small
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 3.785
H-Index - 236
eISSN - 1613-6829
pISSN - 1613-6810
DOI - 10.1002/smll.201804549
Subject(s) - capillary action , surface tension , wetting , materials science , dispersity , nanotechnology , composite material , chemical engineering , physics , engineering , thermodynamics , polymer chemistry
Understanding the mechanical stability of granular‐armored liquid marbles is prerequisite for their applications including encapsulation, sensors, microreactions, and miniaturized liquid storage. Most liquid marbles are armored with agglomerated granular structure which complicates the wetting and interacting states of particles, hence, impeding one from understanding the effect of granular size on the mechanical stability of marbles. In this work, using a custom‐built platform to examine the liquid marbles armored by a single layer of uniform grains, it is revealed that larger microsized grains produce stronger liquid marble. This finding is attributed to the gravity‐induced capillary attraction which dominates the interaction of particles and provides additional tension to the granular network of the marble surface, which enhances the mechanical stability of marbles. In addition, different granular network structures are formed at the marble surface by using a binary mixture of monodisperse grains, and their effect on the mechanical stability of marbles is explored. The understandings offer important insights for application involving liquid marbles and provides guideline to formulate robust marble‐based products.