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Ultrafast Electron Transfer in Binary Nanoparticle Superlattices under High Pressure
Author(s) -
Cheng Ji-Chao,
Pan Ling-Yun,
Tu Hong-Yu,
Qi Hong-Jian,
Ji Wen-Yu,
Li Fang-Fei,
Wang Ying-Hui,
Xu Shu-Ping,
Men Zhi-Wei,
Cui Tian
Publication year - 2021
Publication title -
physica status solidi (rrl) – rapid research letters
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.786
H-Index - 68
eISSN - 1862-6270
pISSN - 1862-6254
DOI - 10.1002/pssr.202100066
Subject(s) - nanoclusters , superlattice , quantum dot , materials science , electron transfer , heterojunction , nanoparticle , electron , ultrashort pulse , nanotechnology , binary number , chemical physics , condensed matter physics , optoelectronics , chemistry , physics , optics , laser , quantum mechanics , arithmetic , mathematics
The interparticle spacing of a heterostructure is a crucial factor affecting electron transfer (ET) process. Herein, binary nanoparticle superlattices (BNSLs) composed of CdSe/ZnS quantum dots (QDs) and Au nanoclusters (NCs) are prepared. Steady‐state and time‐resolved spectra illustrate that the ET accelerates as the pressure increases because pressure effectively adjusts the interparticle spacing. The results also demonstrate that the trap state of the CdSe/ZnS QDs affects the ET process of BNSLs.

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