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Charge Transfer in Chromium‐Transition Metal Alloys
Author(s) -
Kulakowski K.,
Maksymowicz A. Z.
Publication year - 1985
Publication title -
physica status solidi (b)
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.51
H-Index - 109
eISSN - 1521-3951
pISSN - 0370-1972
DOI - 10.1002/pssb.2221300226
Subject(s) - electron , manganese , charge (physics) , atomic physics , electron transfer , transition metal , range (aeronautics) , alloy , chromium , condensed matter physics , core charge , metal , materials science , transfer (computing) , chemistry , physics , core electron , metallurgy , quantum mechanics , biochemistry , composite material , catalysis , parallel computing , computer science
Abstract The average T ‐matrix approximation is applied for calculations of charge transfer of 3d‐electrons in transition metal alloys. In the dilute limit for Cr‐based alloys the transfer of electrons from Cr produces a surplus of about 1.1 electrons on V sites. Manganese lacks 1.1 3d‐electrons and Fe gives away 2.2 electrons. The values are in reasonable agreement with experimental data. For a concentration c = 0.5 the transfers are about half of the values for the dilute cases: 0.5, —0.5, and —1, respectively. Atomic short range order has only slight influence on the charge transfer. Atomic long range order plays a considerable role and may even change the sign of the transfer when compared with the chaotic alloy case.

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