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Effect of Zr/Gnp hybrid filler on thermal and ablation properties of carbon‐epoxy composites
Author(s) -
Subha Sivakumar,
Sairam Vadapalli Naga Venkata,
Pal Yash
Publication year - 2021
Publication title -
polymer composites
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.577
H-Index - 82
eISSN - 1548-0569
pISSN - 0272-8397
DOI - 10.1002/pc.25854
Subject(s) - materials science , composite material , flexural strength , composite number , scanning electron microscope , thermogravimetry , epoxy , thermal stability , carbon fibers , filler (materials) , char , sintering , pyrolysis , chemical engineering , engineering
In this work, the Zirconia (Zr) particles were coated with graphene nanoplatelets (Gnps) using the wet chemical synthesis process and sintered at 500°C and 900°C. At sintering temperature of 900°C, the Zr coated with 0.25 wt% Gnp fillers exhibited better oxidation resistance. Thus, the carbon epoxy (C‐Ex) composites containing Zr/Gnp, 0.25 wt%, were fabricated by the hand‐layup technique. The prepared composites were characterized by scanning electron microscopy, thermogravimetry analysis (TGA), flexural, and ablation tests. The C‐Ex composites modified with Zr/Gnps fillers showed significant improvement in thermal stability and flexural strength compared with the pristine sample. The composite containing 0.25 wt% Zr/Gnp filler reduced the mass ablation rate to 23%, whereas back‐surface temperature was decreased to 170°C compared with pure C‐Ex composite. The surface morphology of ablated composite samples revealed that the Zr/Gnp produced char droplet spheres on the carbon fibres, which prevented the further oxidation of the matrix and thus improved the ablative performance.

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