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Chemical recycling processes can contribute to a resource‐efficient plastic economy. Herein, a procedure for the iron‐catalyzed hydrogenation of the carbonate function of end‐of‐life polycarbonates under simultaneous depolymerization is presented. The use of a straightforward iron pincer complex leads to high rate of depolymerization of poly(bisphenol A carbonate) and poly(propylene carbonate) yielding the monomers bisphenol A and 1,2‐propanediol, respectively, as products under mild reaction conditions. Furthermore, the iron complex was able to depolymerize polycarbonates containing goods and mixture of plastics containing polycarbonates.

Hydrogenative Depolymerization of End‐of‐Life Polycarbonates by an Iron Pincer Complex