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Concentrated second‐harmonic generation from a single Al‐covered ZnS nanobelt
Author(s) -
Hu Hongbo,
Wang Kai,
Long Hua,
Han Xiaobo,
Chen Jiawei,
Wang Bing,
Lu Peixiang
Publication year - 2017
Publication title -
laser and photonics reviews
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 3.778
H-Index - 116
eISSN - 1863-8899
pISSN - 1863-8880
DOI - 10.1002/lpor.201600263
Subject(s) - materials science , second harmonic generation , nanostructure , wavelength , laser , optoelectronics , coating , signal (programming language) , energy conversion efficiency , second harmonic imaging microscopy , nanotechnology , optics , aluminium , physics , computer science , programming language , metallurgy
Here we report on the hybrid nanostructures where a single ZnS nanobelt was half‐covered with an aluminum (Al) film, which is an ideal platform for studying the second‐harmonic generation (SHG) enhancement effects of the Al coating. It was fabricated by the lift‐off process and allowed for the accurate comparison of the SHG intensity between the Al‐covered and the same bare ZnS nanobelt under consistent test conditions. The results indicate that the Al coating in the hybrid nanostructures not only confines the pumping laser in the ZnS effectively, but also concentrates the emitted SHG signal greatly, increasing the signal collection efficiency. By the combination of these two effects, ∼60 times enhancement of the SHG intensity is achieved at the optimized geometry size (width and thickness) of the ZnS nanobelts. The Al‐based hybrid nanostructures open up new possibilities for low‐cost, highly efficient and directional coherent nanolight sources at short wavelengths.