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Theory of coherent anti‐stokes continuum resonance Raman scattering in diatomic molecules
Author(s) -
Beckmann A.,
Baierl P.,
Kiefer W.
Publication year - 1986
Publication title -
journal of raman spectroscopy
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.748
H-Index - 110
eISSN - 1097-4555
pISSN - 0377-0486
DOI - 10.1002/jrs.1250170122
Subject(s) - diatomic molecule , raman scattering , resonance (particle physics) , raman spectroscopy , atomic physics , coherent anti stokes raman spectroscopy , scattering , physics , molecule , chemistry , molecular physics , quantum mechanics
A theory is presented which describes coherent anti‐Stokes resonance Raman scattering via continuum electronic states of diatomic molecules. It is applied to the dissociative continuum of the bounded B ( 3 Π 0+ u ) state and the continuum of the repulsive 1 Π 1 u state of the iodine molecule. The theory allows numerical calculations of continuum resonance CARS spectra.