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Modelling study on the source contribution to aerosol over the Tibetan Plateau
Author(s) -
Zhao Min,
Dai Tie,
Wang Hao,
Bao Qing,
Liu Yimin,
Shi Guangyu
Publication year - 2021
Publication title -
international journal of climatology
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.58
H-Index - 166
eISSN - 1097-0088
pISSN - 0899-8418
DOI - 10.1002/joc.7017
Subject(s) - aerosol , environmental science , atmospheric sciences , plateau (mathematics) , climatology , atmosphere (unit) , relative humidity , wind speed , radiative transfer , meteorology , geography , geology , mathematical analysis , mathematics , physics , quantum mechanics
Understanding the source of atmospheric aerosol is an essential step in determining the aerosol radiative effect over the Tibetan Plateau (TP). This study aims to clarify the contributions of anthropogenic and natural emission to the aerosols (carbonaceous and sulphate) characteristics inside the TP. An aerosol model named Spectral Radiation Transport Model for Aerosol Species (SPRINTARS) recently coupled to the climate model named Chinese Academy of Sciences Flexible Global Ocean Atmosphere Land System (CAS‐FGOALS‐f3‐L) is used to simulate meteorological conditions and aerosols from 1985 to 2013, given emissions from the sixth phase of the Coupled Models Intercomparison Project (CMIP6). Comparisons between the simulations and ERA5 reanalysis data present that the model can capture the key spatial and temporal features of meteorological elements (2‐m temperature, relative humidity, and wind field at 500 hPa) over the Asia. Subsequently, we conduct six sensitivity studies to quantify the contributions of sources to aerosol surface concentration, burden and aerosol optical depth (AOD) over the TP. Our results illustrate that the outside and local anthropogenic sources contribute about 75.2% (78.9% in summer and 66.6% in winter) and 13.5% (7.4% in summer and 24.0% in winter) to the annual mean aerosols surface concentrations over the TP. The outside anthropogenic sources contribute to AODs in TP up to 87.3% (93.9% in autumn and 80.6% in winter). The ascending air over the TP is conducive to the transportation of the outsource pollutions to the TP. The outside natural sources (refer to biomass burning sources) contribute about 10% to aerosols over TP, and the inside natural sources play minor roles. The black carbon, organic carbon and sulphate (BOCS) induce average radiative forcing of −0.7 W m −2 at the near surface over the TP.