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HCFC‐22 emissions at global and regional scales between 1995 and 2010: Trends and variability
Author(s) -
Fortems‒Cheiney A.,
Chevallier F.,
Saunois M.,
Pison I.,
Bousquet P.,
Cressot C.,
Wang H. J.,
Yokouchi Y.,
Artuso F.
Publication year - 2013
Publication title -
journal of geophysical research: atmospheres
Language(s) - English
Resource type - Journals
eISSN - 2169-8996
pISSN - 2169-897X
DOI - 10.1002/jgrd.50544
Subject(s) - environmental science , climatology , montreal protocol , inversion (geology) , ozone , atmospheric sciences , seasonality , atmospheric research , greenhouse gas , meteorology , geography , ozone layer , mathematics , statistics , geology , paleontology , oceanography , structural basin
HCFC‒22 (CHClF 2 , chlorodifluoromethane) is an ozone‒depleting substance, the consumption of which is controlled under the Montreal Protocol. Within a Bayesian inversion framework, we use measurements of HCFC‒22 atmospheric concentrations to constrain estimates of HCFC‒22 emissions, at the grid point 3.75°×2.5° and 8 day resolution, from January 1995 to December 2010. Starting from a new gridded bottom‒up inventory which is then optimized, our method shows continuously rising global emissions, from 182±11 Gg in 1995 to the maximum of 410±9 Gg in 2009. This is mainly due to an increase of emissions in developing regions, particularly in Eastern Asia, and occurs despite the current phase‒out in developed countries. The high temporal resolution of our inversion (8 day) allows to reveal some of the emission seasonality, the global posterior sources ranging from 25 Gg/month in November to 42 Gg/month in July, for example, in 2010.