Theory of the radiative lifetime of the  3  B  1  state of SO 2 | Zendy

Phillips Philip | Zendy; Davidson Ernest R. | Zendy

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Theory of the radiative lifetime of the 3 B 1 state of SO 2

Author(s) -

Phillips Philip,

Davidson Ernest R.

Publication year - 1983

Publication title -

journal of computational chemistry

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 0.907

H-Index - 188

eISSN - 1096-987X

pISSN - 0192-8651

DOI - 10.1002/jcc.540040308

Subject(s) - radiative transfer , perturbation theory (quantum mechanics) , atomic physics , physics , collision , radiative equilibrium , phosphorescence , quantum mechanics , fluorescence , computer security , computer science

Interchange and many‐body perturbation theory are applied to the calculation of the radiative lifetime of the 3 B 1 state of SO 2 . The radiative lifetime of 3 B 1 SO 2 is predicted to be 7.6 msec, in excellent agreement with the experimental collision‐free phosphorescence lifetime. As a separate calculation, interchange perturbation theory is used to determine the radiative lifetime of the 1 A 1 state of CH 2 .

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