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Using synthetic tracers as a proxy for summertime PM 2.5 air quality over the Northeastern United States in physical climate models
Author(s) -
Fang Yuanyuan,
Fiore Arlene M.,
Lamarque JeanFrançois,
Horowitz Larry W.,
Lin Meiyun
Publication year - 2013
Publication title -
geophysical research letters
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 2.007
H-Index - 273
eISSN - 1944-8007
pISSN - 0094-8276
DOI - 10.1002/grl.50162
Subject(s) - environmental science , climate change , climate model , climatology , climate sensitivity , aerosol , atmospheric sciences , particulates , air quality index , proxy (statistics) , acid deposition , meteorology , geography , geology , chemistry , oceanography , organic chemistry , soil science , soil water , machine learning , computer science
Fine particulate matter (PM 2.5 ) is a criteria pollutant. Its sensitivity to meteorology implies its distribution will likely change with climate shifts. Limited availability of global climate models with full chemistry complicates efforts to assess rigorously the uncertainties in the PM 2.5 response to a warming climate. We evaluate the potential for PM 2.5 distributions in a chemistry‐climate model under current‐day and warmer climate conditions over the Northeastern United States to be represented by a Synthetic Aerosol tracer (SAt). The SAt implemented into the Geophysical Fluid Dynamics Laboratory chemistry‐climate model (AM3) follows the protocol of a recent multimodel community effort (HTAP), with CO emissions, 25‐day chemical lifetime, and wet deposition rate of sulfate. Over the Northeastern United States, the summer daily time series of SAt correlates strongly with that of PM 2.5 , with similar cumulative density functions under both present and future climate conditions. With a linear regression model derived from PM 2.5 and SAt in the current‐day simulation, we reconstruct both the current‐day and future PM 2.5 daily time series from the simulated SAt. This reconstruction captures the summer mean PM 2.5 , the incidence of days above the 24‐h mean PM 2.5 NAAQS, and PM 2.5 responses to climate change. This reconstruction also works over other polluted Northern Hemispheric regions and in spring. Our proof‐of‐concept study demonstrates that simple tracers can be developed to mimic PM 2.5 , including its response to climate change, as an easy‐to‐implement and low‐cost addition to physical climate models that should help air quality managers to reap the benefits of climate models that have no chemistry.

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