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Atmospheric Deposition of Coal‐Related Pollutants in the Pacific Northwest of the United States from 1950 to 2016
Author(s) -
Sousa Matthew,
Benson Bryce,
Welty Connor,
Price Dylan,
Thirkill Ruth,
Erickson William,
Cummings Mackenzie,
Dunnivant Frank M.
Publication year - 2020
Publication title -
environmental toxicology and chemistry
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.1
H-Index - 171
eISSN - 1552-8618
pISSN - 0730-7268
DOI - 10.1002/etc.4635
Subject(s) - mercury (programming language) , pollutant , coal , environmental science , ice core , deposition (geology) , glacier , sediment , snow , environmental chemistry , oceanography , geology , physical geography , archaeology , ecology , chemistry , geography , paleontology , computer science , programming language , geomorphology , biology
Coal‐related elements are toxic and persistent pollutants that have spread globally since the industrial revolution, mainly from point‐source emissions. A sediment core was collected from Deep Lake in northeastern Washington State (USA) by the Washington State Department of Ecology, with the aim of assessing recent changes in atmospheric deposition in the US Pacific Northwest. The core was divided into depth intervals and dated by lead‐210. A sample from each cross section was digested and analyzed for toxic metals and metalloids using inductively coupled plasma–mass spectrometry. Data show recent increases in the concentrations of arsenic, barium, selenium, and mercury. Comparison with 1993 US Geological Survey ice core data from the Upper Fremont Glacier in Wyoming (USA), Asian coal consumption data, and weather patterns suggests that pollutant inputs to Deep Lake sediments are the result of coal‐burning activities in the Asia–Pacific region. Most notably, mercury deposition in Deep Lake has increased from approximately 20 ppb in 1996 to 9470 ppb in 2014 (an ~400‐fold increase), and since 1993 when the ice core was analyzed. Environ Toxicol Chem 2020;39:335–342. © 2019 SETAC

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