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Size distribution and filtration property of particles generated from laser ablation decontamination process
Author(s) -
Jung ChongHun,
Park HyunSeol,
Won HuiJun,
Moon JeiKwon,
Choi ByungSeon,
Choi WangKyu
Publication year - 2013
Publication title -
environmental progress and sustainable energy
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.495
H-Index - 66
eISSN - 1944-7450
pISSN - 1944-7442
DOI - 10.1002/ep.11679
Subject(s) - filtration (mathematics) , human decontamination , laser ablation , contamination , materials science , fluence , particle (ecology) , particle size , ablation , filter (signal processing) , particle size distribution , laser , analytical chemistry (journal) , ion , chemistry , chromatography , waste management , optics , aerospace engineering , oceanography , computer science , engineering , biology , mathematics , ecology , computer vision , statistics , physics , organic chemistry , geology
This study investigated the size distribution of particles generated from a laser ablation process applied for the decontamination of a hot cell contaminated with radionuclides. To simulate the hot cell contamination conditions, a stainless steel 304 (STS 304) plate on which Co and Cs ions (water soluble radionuclides, WSRs) were deposited and STS 304 specimens coated with Eu 2 O 3 and CeO 2 (water insoluble radionuclides, WIRs) were prepared. The particle size distribution and concentration for each contamination condition were then measured. In addition, the filtration characteristics of the particles produced from the laser ablation processes were examined using a high efficiency air (HEPA) filter to completely remove these particles. Under the same laser ablation conditions, the particle concentrations for the water insoluble‐contaminated specimen were higher than those for the water soluble‐contaminated specimen. The mobility diameter of particles showing the highest concentration ranged from 70 to 80 nm for all tests. For the specimens contaminated with Cs ion, when a potassium salt such as KNO 3 or KOH was added, the concentration of particles generated under the same fluence increased owing to a removal in the form of Cs oxide, such as Cs 2 O. The overall collection efficiency of the tested HEPA filter for the particles generated from the laser ablation was over 99.4% regardless of the type of contaminated specimen. Consequently, it was confirmed that a high efficiency air filter is very effective as a means to capture particles produced from the hot cell decontamination process using laser ablation technique. © 2012 American Institute of Chemical Engineers Environ Prog, 32: 649–654, 2013