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I 2 Promoted Synthesis of 2‐Aminothiadiazoles Employing KSCN as a Sulfur Source Under Metal‐Free Conditions
Author(s) -
Zhu Fuyuan,
Yan Zhaohua,
Ai Chengmei,
Wang Yanmei,
Lin Sen
Publication year - 2019
Publication title -
european journal of organic chemistry
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.825
H-Index - 155
eISSN - 1099-0690
pISSN - 1434-193X
DOI - 10.1002/ejoc.201901250
Subject(s) - chemistry , potassium thiocyanate , sulfur , thiocyanate , aldehyde , hydrazide , potassium , organic chemistry , metal , combinatorial chemistry , inorganic chemistry , catalysis
A new three‐component strategy from aldehyde, p ‐toluenesulfonyl hydrazide and potassium thiocyanate for the synthesis of 2‐aminothiadiazoles promoted by I 2 under metal‐free conditions has been described. Potassium thiocyanate was used as an odorless and low‐toxicity sulfur source. A wide range of aromatic aldehydes can smoothly undergo the three‐component cyclization reaction under the optimized conditions to give the corresponding products in moderate to good yields.

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