Cobalta‐Electrocatalyzed C−H Activation in Biomass‐Derived Glycerol: Powered by Renewable Wind and Solar Energy | Zendy

Meyer Tjark H. | Zendy; Chesnokov Gleb A. | Zendy; Ackermann Lutz | Zendy

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Cobalta‐Electrocatalyzed C−H Activation in Biomass‐Derived Glycerol: Powered by Renewable Wind and Solar Energy

Author(s) -

Meyer Tjark H.,

Chesnokov Gleb A.,

Ackermann Lutz

Publication year - 2020

Publication title -

chemsuschem

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 2.412

H-Index - 157

eISSN - 1864-564X

pISSN - 1864-5631

DOI - 10.1002/cssc.202000057

Subject(s) - renewable energy , electrocatalyst , biomass (ecology) , catalysis , chemistry , renewable resource , solvent , electrochemistry , environmental science , resource (disambiguation) , glycerol , green chemistry , solar energy , chemical engineering , reaction mechanism , organic chemistry , electrode , computer science , engineering , oceanography , geology , electrical engineering , computer network

Aqueous glycerol was identified as a renewable reaction medium for metalla‐electrocatalyzed C−H activation powered by sustainable energy sources. The renewable solvent was employed for cobalt‐catalyzed C−H/N−H functionalizations under mild conditions. The cobalta‐electrocatalysis manifold occurred with high levels of chemo‐ and positional selectivity and allowed for electrochemical C−H activations with broad substrate scope. The resource economy of this strategy was considerably substantiated by the direct use of renewable solar and wind energy.

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