Hybrid Technologies for an Enhanced Carbon Recycling Based on the Enzymatic Reduction of CO 2  to Methanol in Water: Chemical and Photochemical NADH Regeneration | Zendy

Dibenedetto Angela | Zendy; Stufano Paolo | Zendy; Macyk Wojciech | Zendy; Baran Tomasz | Zendy; Fragale Carlo | Zendy; Costa Mirco | Zendy; Aresta Michele | Zendy

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Hybrid Technologies for an Enhanced Carbon Recycling Based on the Enzymatic Reduction of CO 2 to Methanol in Water: Chemical and Photochemical NADH Regeneration

Author(s) -

Dibenedetto Angela,

Stufano Paolo,

Macyk Wojciech,

Baran Tomasz,

Fragale Carlo,

Costa Mirco,

Aresta Michele

Publication year - 2012

Publication title -

chemsuschem

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 2.412

H-Index - 157

eISSN - 1864-564X

pISSN - 1864-5631

DOI - 10.1002/cssc.201100484

Subject(s) - sodium dithionite , chemistry , methanol , photocatalysis , photochemistry , carbon fibers , dithionite , enzyme , irradiation , molar ratio , redox , artificial photosynthesis , nuclear chemistry , inorganic chemistry , organic chemistry , catalysis , materials science , physics , nuclear physics , composite number , composite material

Rocking chair enzyme: Chemical reducing agents (sodium dithionite) or bioglycerol (as H and e − ‐donor under irradiation in the presence of ZnS‐A as photocatalyst) are able to back‐convert NADP + into NADPH, which is used as e − ‐donor in the enzymatic reduction of CO 2 into CH 3 OH. In doing so, the molar ratio CH 3 OH/CO 2 has been increased (without recycling of NADP + ) using the photocatalyst.

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