On the Nature of the Active Site for the Oxidative Amination of Benzene to Aniline over NiO/ZrO 2  as Cataloreactant | Zendy

Hoffmann Nora | Zendy; Löffler Elke | Zendy; Breuer Niklas A. | Zendy; Muhler Martin | Zendy

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On the Nature of the Active Site for the Oxidative Amination of Benzene to Aniline over NiO/ZrO 2 as Cataloreactant

Author(s) -

Hoffmann Nora,

Löffler Elke,

Breuer Niklas A.,

Muhler Martin

Publication year - 2008

Publication title -

chemsuschem

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 2.412

H-Index - 157

eISSN - 1864-564X

pISSN - 1864-5631

DOI - 10.1002/cssc.200700130

Subject(s) - aniline , amination , benzene , chemistry , microreactor , non blocking i/o , ammonia , inorganic chemistry , adsorption , reductive amination , photochemistry , catalysis , organic chemistry

Suspended amination : Semi‐batch oxidative synthesis of aniline from benzene and ammonia was performed at atmospheric pressure using a NiO/ZrO 2 cataloreactant in a microreactor flow setup. A Langmuir–Hinshelwood mechanism is suggested based on the surface reaction between adsorbed benzene‐ and ammonia‐derived NH x species on metallic Ni surface sites.

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