Sunlight‐Driven Synthesis of 1,2,4‐Thiadiazoles via Oxidative Construction of a Nitrogen‐Sulfur Bond Catalyzed by a Reusable Covalent Organic Framework | Zendy

Yuan Jiangpei | Zendy; Xia Qiangqiang | Zendy; Zhu Weiwei | Zendy; Wu Cunluo | Zendy; Wang Bingxin | Zendy; Liu Baoying | Zendy; Yang Xiaobo | Zendy; Xu Yuanqing | Zendy; Xu Hao | Zendy

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Sunlight‐Driven Synthesis of 1,2,4‐Thiadiazoles via Oxidative Construction of a Nitrogen‐Sulfur Bond Catalyzed by a Reusable Covalent Organic Framework

Author(s) -

Yuan Jiangpei,

Xia Qiangqiang,

Zhu Weiwei,

Wu Cunluo,

Wang Bingxin,

Liu Baoying,

Yang Xiaobo,

Xu Yuanqing,

Xu Hao

Publication year - 2020

Publication title -

chemphotochem

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.13

H-Index - 18

ISSN - 2367-0932

DOI - 10.1002/cptc.201900263

Subject(s) - covalent bond , thiadiazoles , sulfur , chemistry , catalysis , photochemistry , nitrogen , organic synthesis , oxidative phosphorylation , sunlight , organic chemistry , combinatorial chemistry , biochemistry , physics , astronomy

Employing a two‐dimensional covalent organic framework as the reusable solar photosensitizer, the sunlight‐driven aerobic oxidative construction of a nitrogen‐sulfur bond has been achieved. 3,5‐Disubstituted 1,2,4‐thiadiazoles are smoothly prepared in water by using this procedure. Furthermore, a radical mechanism with a sunlight‐promoted single electron transfer (SET) process is proposed for this transformation.

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