An Electron Dynamics Mechanism of Charge Separation in the Initial‐Stage Dynamics of Photoinduced Water Splitting in XMnWater (X=OH, OCaH) and Electron–Proton Acceptors | Zendy

Yamamoto Kentaro | Zendy; Takatsuka Kazuo | Zendy

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An Electron Dynamics Mechanism of Charge Separation in the Initial‐Stage Dynamics of Photoinduced Water Splitting in XMnWater (X=OH, OCaH) and Electron–Proton Acceptors

Author(s) -

Yamamoto Kentaro,

Takatsuka Kazuo

Publication year - 2015

Publication title -

chemphyschem

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.016

H-Index - 140

eISSN - 1439-7641

pISSN - 1439-4235

DOI - 10.1002/cphc.201500416

Subject(s) - excited state , chemistry , proton , electron , water splitting , photoinduced charge separation , cluster (spacecraft) , electron transfer , ammonia , doping , chemical physics , photochemistry , inorganic chemistry , atomic physics , materials science , artificial photosynthesis , photocatalysis , catalysis , physics , biochemistry , optoelectronics , organic chemistry , quantum mechanics , computer science , programming language

An electron dynamics mechanism of charge separation in the initial stage of excited‐state reactions of the class of XMnOH 2 ⋅⋅⋅A ${ \to }$ XMnOH⋅⋅⋅HA (X=OH or OCaH; A= N ‐methylformamidine, guanidine, imidazole, or ammonia cluster) is reported. The dynamic effect of calcium doping is also revealed. This study provides a novel factor to be considered in designing efficient systems for photoinduced water splitting.

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