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Dimensional effect of graphite flow field channels of a direct methanol fuel cell under different operating conditions
Author(s) -
Tan Zhenhao,
Wang Aoyu,
Yuan Wei,
Han Fuchang,
Ye Guangzhao,
Xia Hongrong,
Tang Yong
Publication year - 2018
Publication title -
the canadian journal of chemical engineering
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.404
H-Index - 67
eISSN - 1939-019X
pISSN - 0008-4034
DOI - 10.1002/cjce.22995
Subject(s) - anode , cathode , direct methanol fuel cell , volumetric flow rate , methanol , materials science , oxygen , methanol fuel , graphite , chemical engineering , analytical chemistry (journal) , nuclear engineering , chemistry , composite material , electrode , mechanics , chromatography , engineering , organic chemistry , physics
Direct methanol fuel cells are a potential candidate to replace traditional power sources for portable applications. The flow field design, manufacture, and optimization are of great significance to the cell performance. When the scale of flow channels decreases to the level of submillimeter‐scale, it is favourable to the reactant and product management. This paper focuses on the effectiveness of using a multi‐tooth planing technique to create submillimeter‐scale parallel channels in a graphite sheet. Besides the structural parameters of flow channels, a series of operating parameters are experimentally investigated, including methanol concentration, methanol feed rate, oxygen feed rate, cathode backpressure, and environmental temperature. Results indicate that the prepared channels promote a higher cell performance than the traditional design with a larger scale. It is beneficial to both the anode and cathode performances, but it has a more prominent effect at the anode. The methanol concentration of 4 mol/L yields the best performance. Using a relatively lower methanol feed rate below 0.5 mL/min has a more obvious effect on the fuel cell. The cell performance is insensitive to the change of cathode oxygen feed rate and backpressure especially when the oxygen can be sufficiently supplied. In this case we can use lower levels of oxygen feed rate and cathode backpressure. The cell temperatures and influence of environmental temperature are also discussed.