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Tuning Interfacial Structures for Better Catalysis of Water Electrolysis
Author(s) -
Xiang Rui,
Peng Lishan,
Wei Zidong
Publication year - 2019
Publication title -
chemistry – a european journal
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.687
H-Index - 242
eISSN - 1521-3765
pISSN - 0947-6539
DOI - 10.1002/chem.201901168
Subject(s) - electrolysis of water , electrolysis , interface (matter) , nanotechnology , durability , design elements and principles , catalysis , computer science , materials science , biochemical engineering , process engineering , chemistry , engineering , electrode , biochemistry , software engineering , electrolyte , bubble , database , maximum bubble pressure method , parallel computing
Interface modulation, as an old concept of heterogeneous catalysis, represents an emerging, fast‐growing and exciting direction in the field of water electrolysis. Over the past five years, diverse hetero‐nanostructures have been synthesised as water electrolysis catalysts by taking advantage of interface modulation. However, it seems that the performance (i.e., efficiency and durability) of these materials needs to be further improved. Therefore, a comprehensive summary of recent achievements and the challenging issues concerning the regulation of material functionalities through interface modulation is necessary and helpful. Herein, firstly, the fundamentals of water electrolysis are outlined, and then the delicate design and fine control of well‐defined interfaces, as well as related mechanisms for performance improvement are discussed. Finally, future opportunities and challenges in the everlasting pursuit of highly efficient and robust water electrolysis catalysts are highlighted.

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