A Multifunctional Magnetic Material under Pressure | Zendy

RodríguezVelamazán J. Alberto | Zendy; Fabelo Oscar | Zendy; Beavers Christine M. | Zendy; Natividad Eva | Zendy; Evangelisti Marco | Zendy; Roubeau Olivier | Zendy

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A Multifunctional Magnetic Material under Pressure

Author(s) -

RodríguezVelamazán J. Alberto,

Fabelo Oscar,

Beavers Christine M.,

Natividad Eva,

Evangelisti Marco,

Roubeau Olivier

Publication year - 2014

Publication title -

chemistry – a european journal

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.687

H-Index - 242

eISSN - 1521-3765

pISSN - 0947-6539

DOI - 10.1002/chem.201402046

Subject(s) - antiferromagnetism , magnetometer , ambient pressure , spin crossover , neutron diffraction , condensed matter physics , materials science , spin (aerodynamics) , diffraction , atmospheric temperature range , nuclear magnetic resonance , physics , thermodynamics , magnetic field , optics , quantum mechanics

Fe II (Metz) 6 ](Fe III Br 4 ) 2 (Metz=1‐methyltetrazole) is one of the rare systems combining spin‐crossover and long‐range magnetic ordering. A joint neutron and X‐ray diffraction and magnetometry study allows determining its collinear antiferromagnetic structure, and shows an increase of the Néel temperature from 2.4 K at ambient pressure, to 3.9 K at 0.95 GPa. Applied pressure also enables a full high‐spin to low‐spin switch at ambient temperature.

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