Nanoconfinement and Catalytic Dehydrogenation of Ammonia Borane by Magnesium‐Metal–Organic‐Framework‐74 | Zendy

Gadipelli Srinivas | Zendy; Ford Jamie | Zendy; Zhou Wei | Zendy; Wu Hui | Zendy; Udovic Terrence J. | Zendy; Yildirim Taner | Zendy

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Nanoconfinement and Catalytic Dehydrogenation of Ammonia Borane by Magnesium‐Metal–Organic‐Framework‐74

Author(s) -

Gadipelli Srinivas,

Ford Jamie,

Zhou Wei,

Wu Hui,

Udovic Terrence J.,

Yildirim Taner

Publication year - 2011

Publication title -

chemistry – a european journal

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.687

H-Index - 242

eISSN - 1521-3765

pISSN - 0947-6539

DOI - 10.1002/chem.201100090

Subject(s) - ammonia borane , dehydrogenation , magnesium , borane , catalysis , ammonia , chemistry , chemical engineering , materials science , inorganic chemistry , organic chemistry , engineering

Trapped and released : Ammonia borane (AB) incorporated within the one‐dimensional hexagonal nanopores of magnesium‐metal–organic‐framework‐74 shows clean and exceptionally improved H 2 ‐release properties when compared to pristine AB (see figure; C gray, O red, Mg green, H white, N blue, B orange). In this system, the kinetics and the temperature of AB dehydrogenation can be easily tuned.

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