Dynamics of the Delocalized Charges of a Radical Anion in A⋅T DNA Duplexes | Zendy

Yamagami Ryuhei | Zendy; Kobayashi Kazuo | Zendy; Tagawa Seiichi | Zendy

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Dynamics of the Delocalized Charges of a Radical Anion in A⋅T DNA Duplexes

Author(s) -

Yamagami Ryuhei,

Kobayashi Kazuo,

Tagawa Seiichi

Publication year - 2009

Publication title -

chemistry – a european journal

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.687

H-Index - 242

eISSN - 1521-3765

pISSN - 0947-6539

DOI - 10.1002/chem.200902080

Subject(s) - delocalized electron , microsecond , unpaired electron , ion , charge (physics) , chemistry , electron , adduct , electron transfer , transient (computer programming) , dna , photochemistry , chemical physics , crystallography , physics , optics , quantum mechanics , computer science , biochemistry , organic chemistry , operating system

Gone in the blink of any eye : The transient spectrum of the electron adducts of A⋅T pairs initially obtained shows that the unpaired electron is localized to the A site (see picture). Subsequently charge transfer from transients (A⋅T) .− to T .− occurs over the time range of microseconds.

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