Conversion of Dinitrogen to Nitriles at a Multinuclear Titanium Framework | Zendy

Guru Murali Mohan | Zendy; Shima Takanori | Zendy; Hou Zhaomin | Zendy

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Conversion of Dinitrogen to Nitriles at a Multinuclear Titanium Framework

Author(s) -

Guru Murali Mohan,

Shima Takanori,

Hou Zhaomin

Publication year - 2016

Publication title -

angewandte chemie international edition

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 5.831

H-Index - 550

eISSN - 1521-3773

pISSN - 1433-7851

DOI - 10.1002/anie.201607426

Subject(s) - chemistry , aldehyde , diimide , nitro , surface modification , titanium , ammonia , combinatorial chemistry , nitrile , functional group , polymer chemistry , organic chemistry , medicinal chemistry , catalysis , molecule , alkyl , perylene , polymer

Activation and functionalization of N 2 : A mixed diimide/dinitride tetranuclear titanium complex formed by activation of dinitrogen served as a unique platform for the synthesis of nitriles (see picture). Functional groups such as aromatic C−X (X=Cl, Br, I) bonds, nitro groups, and ammonia‐sensitive aldehyde and chloromethyl moieties were compatible with the synthetic method.

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