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Metalloenzyme‐Like Zeolites as Lewis Acid Catalysts for CC Bond Formation
Author(s) -
Van de Vyver Stijn,
RománLeshkov Yuriy
Publication year - 2015
Publication title -
angewandte chemie international edition
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 5.831
H-Index - 550
eISSN - 1521-3773
pISSN - 1433-7851
DOI - 10.1002/anie.201503701
Subject(s) - catalysis , lewis acids and bases , chemistry , organic chemistry
The use of metalloenzyme‐like zeolites as Lewis acid catalysts for CC bond formation reactions has received increasing attention over the past few years. In particular, the observation of direct aldol condensation reactions enabled by hydrophobic zeolites with isolated framework metal sites has encouraged the development of catalytic approaches for producing chemicals from biomass‐derived compounds. The discovery of new Diels–Alder cycloaddition/dehydration routes and experimental and computational studies of Lewis acid catalyzed carbonyl–ene reactions have given a further boost to this rapidly evolving field.

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