Radical CH Functionalization of Heteroarenes under Electrochemical Control | Zendy

O'Brien Alexander G. | Zendy; Maruyama Akinobu | Zendy; Inokuma Yasuhide | Zendy; Fujita Makoto | Zendy; Baran Phil S. | Zendy; Blackmond Donna G. | Zendy

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Radical CH Functionalization of Heteroarenes under Electrochemical Control

Author(s) -

O'Brien Alexander G.,

Maruyama Akinobu,

Inokuma Yasuhide,

Fujita Makoto,

Baran Phil S.,

Blackmond Donna G.

Publication year - 2014

Publication title -

angewandte chemie international edition

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 5.831

H-Index - 550

eISSN - 1521-3773

pISSN - 1433-7851

DOI - 10.1002/anie.201407948

Subject(s) - surface modification , electrochemistry , chemistry , combinatorial chemistry , radical , peroxide , organic chemistry , electrode

Electrochemical reactions are shown to be effective for the CH functionalization of a number of heterocyclic substrates that are recalcitrant to conventional peroxide radical initiation conditions. Monitoring reaction progress under electrochemical conditions provides mechanistic insight into the CH functionalization of a series of heterocycles of interest in medicinal chemistry.

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