Ultrafast Solvent‐Assisted Electronic Level Crossing in 1‐Naphthol | Zendy

Messina Fabrizio | Zendy; PrémontSchwarz Mirabelle | Zendy; Braem Olivier | Zendy; Xiao Dequan | Zendy; Batista Victor S. | Zendy; Nibbering Erik T. J. | Zendy; Chergui Majed | Zendy

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Ultrafast Solvent‐Assisted Electronic Level Crossing in 1‐Naphthol

Author(s) -

Messina Fabrizio,

PrémontSchwarz Mirabelle,

Braem Olivier,

Xiao Dequan,

Batista Victor S.,

Nibbering Erik T. J.,

Chergui Majed

Publication year - 2013

Publication title -

angewandte chemie international edition

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 5.831

H-Index - 550

eISSN - 1521-3773

pISSN - 1433-7851

DOI - 10.1002/anie.201301931

Subject(s) - ultrashort pulse , femtosecond , excited state , solvent , spectroscopy , computer science , photochemistry , dimethyl sulfoxide , internal conversion , chemistry , information retrieval , physics , organic chemistry , atomic physics , optics , quantum mechanics , laser , spectral line

Solvent effects : The nonadiabatic inversion dynamics of the energetic order of the electronic excited states of the photoacid 1‐naphthol have been revealed by ultrafast spectroscopy on a femtosecond timescale (see picture; IC=internal conversion). The energetic order of the excited states L a and L b of 1‐naphthol is reversed in 60 fs in polar dimethyl sulfoxide solvent.

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